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Removing members from a contact group is as easy as adding them, but on the Samsung device, you must select the edit mode to remove members.

Android 11 | One UI 3.0
Step 1: Tap on  Contacts
Step 2: Open the  Menu
Step 3: Choose a  Group
Step 4: Tap on  Edit
Step 5: Remove the desired  Member  and tap  Save
  1. Tap on Contacts
  2. Open the Menu
  3. Choose a Group
  4. Tap on Edit
  5. Remove the desired Member and tap Save
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Samsung Instructions